Production of geranylgeraniol on overexpression of a prenyl diphosphate synthase fusion gene in Saccharomyces cerevisiae.
An acyclic diterpene alcohol, (E,E,E)-geranylgeraniol (GGOH), is one of the important compounds used as perfume and pharmacological agents. A deficiency of squalene (SQ) synthase activity allows yeasts to accumulate an acyclic sesquiterpene alcohol, (E,E)-farnesol, in their cells. Since sterols are essential for the growth of yeasts, a deficiency of SQ ... synthase activity makes the addition of supplemental sterols to the culture media necessary. To develop a GGOH production method not requiring any supplemental sterols, we overexpressed HMG1 encoding hydroxymethylglutaryl-CoA reductase and the genes of two prenyl diphosphate synthases, ERG20 and BTS1, in Saccharomyces cerevisiae. A prototrophic diploid coexpressing HMG1 and the ERG20-BTS1 fusion accumulated GGOH with neither disruption of the SQ synthase gene nor the addition of any supplemental sterols. The GGOH content on the diploid cultivation in a 5-l jar fermenter reached 138.8 mg/l under optimal conditions.
Mesh Terms:
Cell Adhesion Molecules, Eremothecium, Fungal Proteins, Gene Expression Regulation, Fungal, Promoter Regions, Genetic, Saccharomyces cerevisiae Proteins, Transcription Factors
Cell Adhesion Molecules, Eremothecium, Fungal Proteins, Gene Expression Regulation, Fungal, Promoter Regions, Genetic, Saccharomyces cerevisiae Proteins, Transcription Factors
Appl. Microbiol. Biotechnol.
Date: Jul. 01, 2010
PubMed ID: 20393702
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