Role of Saccharomyces cerevisiae oxidoreductases Bdh1p and Ara1p in the metabolism of acetoin and 2,3-butanediol.
NAD-dependent butanediol dehydrogenase (Bdh1p) from Saccharomyces cerevisiae reversibly transforms acetoin to 2,3-butanediol in a stereospecific manner. Deletion of BDH1 resulted in an accumulation of acetoin and a diminution of 2,3-butanediol in two S. cerevisiae strains under two different growth conditions. The concentrations of (2R,3R)-2,3-butanediol are mostly dependent on Bdh1p activity, ... while those of (meso)-2,3-butanediol are also influenced by the activity of NADP(H)-dependent oxidoreductases. One of them has been purified and shown to be d-arabinose dehydrogenase (Ara1p), which converts (R/S)-acetoin to meso-2,3-butanediol and (2S,3S)-2,3-butanediol. Deletion of BDH2, a gene adjacent to BDH1, whose encoded protein is 51% identical to Bdh1p, does not significantly alter the levels of acetoin or 2,3-butanediol in comparison to the wild-type strain. Furthermore, we have expressed Bdh2p with a histidine tag and have shown it to be inactive toward 2,3-butanediol. A whole-genome expression analysis with microarrays demonstrates that BDH1 and BDH2 are reciprocally regulated.
Mesh Terms:
Acetoin, Aerobiosis, Alcohol Oxidoreductases, Amino Acid Substitution, Anaerobiosis, Butylene Glycols, Cloning, Molecular, Conserved Sequence, Fermentation, Gene Deletion, Genetic Engineering, Hydrogen-Ion Concentration, Kinetics, Mutation, NAD, Oxidoreductases, Saccharomyces cerevisiae, Saccharomyces cerevisiae Proteins, Sequence Alignment, Substrate Specificity, Sugar Alcohol Dehydrogenases
Acetoin, Aerobiosis, Alcohol Oxidoreductases, Amino Acid Substitution, Anaerobiosis, Butylene Glycols, Cloning, Molecular, Conserved Sequence, Fermentation, Gene Deletion, Genetic Engineering, Hydrogen-Ion Concentration, Kinetics, Mutation, NAD, Oxidoreductases, Saccharomyces cerevisiae, Saccharomyces cerevisiae Proteins, Sequence Alignment, Substrate Specificity, Sugar Alcohol Dehydrogenases
Appl. Environ. Microbiol.
Date: Feb. 01, 2010
PubMed ID: 19966022
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